The Melancholy of Haruhi Suzumiya's second ending "Tomare!"
That's how I see it at least as I consider it to be somewhat overshadowed by the first ending "Hare Hare Yukai", I love both and consider them to be equally phenomenal and unique.
TechTv and Anime Unleashed were amazing before G4 ruined it. It was probably the first and only time I ever saw subbed anime on tv. Lain, Boogiepop, Crest of the Stars, SoulTaker and Silent Mobius were amazing to see for the first time.
My favorite Anime intro is Saint Seiya's Pegasus Fantasy for obvious reasons, but my favorite ending is Shurato's Sabaku no Meizu although I prefer the Brazilian version Viajante Dos Sonhos
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